FMR STUDIES OF CrO2 EPITAXIAL THIN FILMS
B.Z. Rameev
1,2, R.Yilgin
1,2, B. Aktas
1,2, and
Lenar.R. Tagirov3 (

)
1Gebze Institute of Technology, P.K. 141, 41400 Gebze-Kocaeli, Turkey.
2A. Gupta
IBM T. J. Watson Research Center, Yorktown Heights, New York 10598, USA
3Kazan State University, 420008 Kazan, Russia.
Epitaxial thin films of (100) CrO2 were fabricated by chemical
vapor deposition (CVD) at
atmospheric oxygen pressure onto (100) TiO2 single-crystal
substrates. The films were 20, 60, 66, 80,
150, and 161 nm in thickness. Ferromagnetic Resonance (FMR) measurements were
performed at X-
band (9.5 GHz) at room temperature for all samples. Angular dependencies of
FMR spectra in both
"in-plane" and "out-of-plane" geometries were measured. The directions of easy
and hard axes of
magnetization were determined from "in-plane" measurements, when the DC
magnetic field was
rotated in the film plane. The orientation of crystallographic axes in the
film plane was controlled by
the X-ray measurements. In the "out-of-plane" measurements, the DC magnetic
field was rotated from
that at room temperature the minimal FMR resonance field (i.e. "easy axis" of
magnetization) in all
films is achieved in the direction of DC magnetic field parallel to the "c"
axis of CrO2 rutile structure.
Splitting (or asymmetric lineshape) of FMR response due to the surface and
bulk modes was observed.
This indicates an essential surface pinning of magnetization at interfaces of
CrO2 films. A shift of
FMR signal to the lower magnetic fields in the normal direction reflecting an
increase of the
anisotropy field was observed upon decrease of the film thickness. The values
of the room temperature
magnetization and anisotropy fields were also estimated from the FMR
measurements. LRT thanks
UR.01.01.061 and NIOKR/ANT 06-6.2-47/2001(F) for partial support.